If you like billiards, Hustle Kings is a good option as you buy it on PS3 you get it on Vita.
For Vita: Super Stardust is crazy good. I liked it a lot more than the PS3 one even.
For PS3: Dead Nation Payday: The Heist Sonic Adventure Killzone 3 Multiplayer Beyond Good and Evil HD Splinter Cells (They might still be on sale, I don't recall) Resident Evil 4 Crysis MAG (not sure how the community is anymore?)
To save our Mother Earth from any alien attack
From vicious giant insects who have once again come back
We'll unleash all our forces we won't cut them any slack
The EDF deploys!!
On the PS3 I've gotten the most out of Might & Magic: Clash of Heroes by far. Killzone 3 Multiplayer is also a great deal. And on my Vita it's the free Motorstorm RC and its expansion packs that I've spent most of my time on.
PS3: Bionic Commando: ReArmed Journey Outland Shatter Super Stardust Dead Nation Klonoa: Door to Phantomile (PS1 Classic) Trine Tales from Space: About a Blob Limbo Joe Danger
Oh, and don't forget about PSP games for your Vita. There are some real classics there, such as Megaman Maverick Hunter X and Lunar: Silver Star Harmony, among many others.
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Topic: Great PSN games for $20 or less
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