The only games that make the most of the Sharp Shooters are SOCOM 4: U.S. Navy SEALs and Killzone 3, and to the best of my knowledge neither support two Move controllers at once.
Greg Hastings Paintball 2 has split-screen multiplayer with Move, but doesn't make use of the Sharp Shooter's reload/variable shooting buttons. Of course you can still use the Sharp Shooter to make you look badass while playing
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Topic: Sharp Shooter Guns PS3
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